高小雅,李旭兵,佟振合,吴骊珠.化学通报,2021,84(1):10-15. |
量子点人工光合成化学转换研究进展 |
Recent Advances in Quantum Dots Based Artificial Photosynthesis |
投稿时间:2020-08-06 修订日期:2020-09-03 |
DOI: |
中文关键词: 量子点 人工光合成 光催化制氢 光催化CO2还原 有机转换 |
英文关键词:Quantum dots Artificial photosynthesis Photocatalytic H2 evolution Photocatalytic CO2 reduction Organic transformation |
基金项目:国家自然科学基金项目(21861132004,21971251,21603248)资助 |
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中文摘要: |
利用半导体量子点为光催化剂通过人工光合成的方式把H2O或CO2转化为H2或CO从而获得氢气或其他太阳能燃料,被认为是解决能源和环境危机的有效途径。量子点由于其独特的光物理和光化学性质(如优异的吸光能力、可调的能带结构、多激子生成、表面丰富的活性位点等)在人工光合成化学转换领域受到了广泛的关注。本文总结了近年来作者团队在量子点人工光合成领域取得的进展,并对该领域的前景进行了展望。 |
英文摘要: |
The facile conversion of H2O or CO2 into chemical fuels (such as H2, CO) via semiconductor quantum dots (QDs) artificial photosynthesis is considered as an effective way to solve the energy and environmental crisis. Due to the unique photophysical and photochemical properties (e.g., excellent light absorption capacity, adjustable energy band structure, multi-exciton generation, abundant surface active sites, etc.), QDs have received much attention in the field of artificial photosynthesis in recent years. Here, we summarize our recent advances in chemical conversions via artificial photosynthesis using semiconductor QDs, and also provide prospects of future studies. |
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