| 邵伟,张晓东.化学通报,2023,86(6):657-664. |
| CO2还原反应二维电催化剂研究进展 |
| Progresses in Two-dimensional Electrocatalysts for CO2 Reduction |
| 投稿时间：2022-12-27 修订日期：2023-02-04 |
| DOI： |
| 中文关键词: 二维材料 电催化 二氧化碳还原 表面缺陷工程 单原子 |
| 英文关键词:Two-dimensional materials, Electrocatalysis, Carbon dioxide reduction, Surface defect engineering, Single atom |
| 基金项目:国家重点研发计划项目(2022YFA1502903)和国家自然科学基金项目(22275179)资助 |
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| 中文摘要: |
| 二氧化碳(CO2)电化学还原为高附加值化学品在解决CO2过量排放上具有极好的应用前景,但这需要开发先进的电催化剂来降低CO2活化能并提高还原产物的选择性。受益于独特的几何结构,二维材料在电催化CO2还原反应中得到了广泛研究。本综述将系统介绍应用于CO2还原反应的二维电催化剂上的最新进展。我们也将揭示特征结构与电催化性能之间的构效关系。我们希望本文可以为开发CO2还原电催化剂提供有益的指导。 |
| 英文摘要: |
| Electrocatalytic CO2 reduction into value-added chemicals holds great potential in solving excessive CO2 emissions, however, advanced electrocatalysts for lowering the activation energy and enhancing selectivity in CO2 reduction are needed. Benefiting from the unique geometrical structures, two-dimensional (2D) materials have been extensively studied in the electrocatalytic CO2 reduction reaction. In this review, we systematically overview the progresses two-dimensional electrocatalysts for CO2 reduction. Meanwhile, we also discuss the structure-activity correlations of electrocatalysts, and we hope that this review can guide the design of electrocatalysts for CO2 reduction. |
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